Beibei Wang, Zhuoyao Lv, Nan Ning, Yichen Zhang, Jiquan Zhang
Accurate prediction of critical temperature, pressure, and volume is essential for thermodynamic modeling and process safety design, yet remains challenging for complex molecules under data-scarce conditions. Here, we develop a multimodal GNN-BERT framework that integrates SMILES-based chemical semantics with two-dimensional topology and three-dimensional molecular geometry for critical property prediction. BERT captures molecular sequence information, while graph neural networks learn topology- and geometry-aware representations through message passing. Evaluation on 913 chemical compounds demonstrates that the proposed framework consistently outperforms conventional machine-learning models and single-modality baselines. Importantly, comparative analyses among BERT, BERT+2D-GNN, and BERT+3D-GNN reveal that incorporating three-dimensional molecular geometry provides a consistent 5-10% improvement across critical temperature, pressure, and volume prediction. Additional validation using random forest and support vector regression further confirms that the predictive contribution of 3D molecular information is not architecture-dependent. These results highlight three-dimensional molecular geometry as an important structural parameter for data-driven critical property prediction and provide a reliable computational strategy for thermodynamic estimation and chemical process safety applications.