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◆ Gels (Basel, Switzerland)2026-08-21

Engineering Parameter Window for Filament Formation and Early-Stage Evolution in Embedded Printing of Gelatin/Alginate Hydrogels Within Carbomer Support Baths.

Jinwei Li, Wang Tang, Zihang Yan, Huansi Mo, Jinhu Wang, Lin Lin, Yong Wang, Hui You, Yuanfen Chen

原始摘要(英文原文)· Original abstract
Embedded 3D printing of hydrophilic hydrogels in aqueous support baths often suffers from filament deformation, positional deviation, and diffusion before complete cross-linking, while practical parameter-selection guidelines for specific material systems remain limited. In this work, an integrated engineering evaluation method was developed to characterize filament formation and early-stage evolution during embedded printing of gelatin/sodium alginate inks in Carbomer support baths. Filament quality was assessed using cross-sectional geometry, contour irregularity, deposition position, and early-stage diffusion ratio. The effects of printing kinematics and material rheology are systematically examined to establish a practical process window for this hydrophilic ink-bath system. The results show that the speed ratio between substrate and ink is a primary factor controlling filament geometry and deposition position, and a ratio close to 1 yields the most balanced cross-sectional morphology without position shift from the printed nozzle. Ink with high viscosity maintains contour irregularity within a narrow range of 0.005-0.009 and suppresses early diffusion, whereas a support bath with high viscosity and ink with high viscosity combination further slows diffusional evolution by about 70%. Based on the identified process window, several three-dimensional hydrogel structures were fabricated successfully. The proposed workflow provides a practical route for process evaluation and parameter selection in hydrophilic embedded printing, especially for continuous filament and tubular structures, and offers engineering guidance for bio-soft material fabrication in applications.
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Engineering Parameter Window for Filament Formation and Early-Stage Evolution in Embedded Printing of Gelatin/Alginate Hydrogels Within Carbomer Support Baths. — 科研速览 Science Skim