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◆ Science Advances2026-03-06· Hexagonal lattice

Spin excitation continuum from degenerate states in the mixed ferro-antiferromagnetic exchange system CeMgAl <sub>11</sub> O <sub>19</sub>

Bin Gao, Tong Chen, Chunxiao Liu, Mason Klemm, Shu Zhang, Zhen Ma, Xianghan Xu, Choongjae Won, Gregory T. McCandless, Karthik Rao, Naoki Murai, Seiko Ohira‐Kawamura, Stephen J. Moxim, Jason T. Ryan, Xiaozhou Huang, Xiaoping Wang, Manh Duc Le, Emilia Morosan, Julia Y. Chan, Sang-Wook Cheong, Oleg Tchernyshyov, Leon Balents, Pengcheng Dai

原始摘要(英文原文)· Original abstract
In the search for unconventional magnetism, exotic quantum states are characterized by a lack of order and a broad spin excitation continuum approaching zero temperature. We study the two-dimensional triangular-lattice effective spin- 1 2 system CeMgAl 11 O 19 , which shows slight disorder but no magnetic ordering down to 100 millikelvin. Spin-wave analysis in the magnetic-field–polarized state determines the spin Hamiltonian featuring a mixed ferromagnetic-antiferromagnetic nearest-neighbor exchange interaction [ J z = −0.024(5) milli–electron volts, J ⊥ = 0.056(3) milli–electron volts]. This places the system near an exactly solvable point of the spin- 1 2 triangular-lattice XXZ model ( J z = − 1 2 J ⊥ ) with extensive ground-state degeneracy. In zero field, neutron spectroscopy reveals a prominent continuum; we show that this arises from an ensemble average of spin-wave spectra across the degenerate ground-state manifold. This demonstrates that the role of weak quenched disorder can be quantitatively constrained: It inhibits unique ground-state selection and stabilizes a local distribution within the degenerate manifold, yielding continuum-like spectra that necessitate a critical reevaluation of the experimental signatures of exotic quantum states.
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Spin excitation continuum from degenerate states in the mixed ferro-antiferromagnetic exchange system CeMgAl <sub>11</sub> O <sub>19</sub> — 科研速览 Science Skim