Layer Edelstein Effect.

Electrical control of magnetism represents a fundamental route toward next-generation spintronic functionalities. In this Letter, we introduce a universal current-induced spin phenomenon in bilayer systems, termed the layer Edelstein effect (LEE), which serves as the natural counterpart of the layer Hall effect in real space. It is defined by the emergence of layer-resolved spin magnetizations with opposite components on the top and bottom layers, driven by an in-plane charge current and controllable by an external electric field. We establish the general existence of the LEE using a minimal bilayer k·p theory. By combining symmetry analysis with a general bilayer stacking framework, we derive a model-independent symmetry criterion demonstrating that the LEE is generically allowed in a broad class of nonmagnetic bilayer stacking systems. We further show that the LEE admits two universal manifestations: explicit layer-opposite spin magnetization components mandated directly by symmetry, and components become activated upon symmetry reduction by external electric fields. First-principles calculations on stacked bilayer MoSSe, MoTe_{2}, and WTe_{2} confirm the predicted effect and illustrate their experimental feasibility. Our Letter establishes the LEE as a generic symmetry-governed response of bilayer systems, providing a unified conceptual framework for electrically generating and manipulating layer-resolved spin polarization.