Jiawei Guo, Chuanshuai Huang, Jinxin Ge, Shengwei Zeng, Zhenyi Weng, Jun Zhang, Mengke Fang, Heyuan Song, Liang Liu, Yunmei Li, Zhiming Pan, Changjian Li, Jingsheng Chen, Xiancong Lu, Weinan Lin
While non-trivial spin-orbit coupling (SOC) was predicted early in high-temperature cuprate superconductors (HTCS), its precise role and microscopic consequences remain unresolved. This challenge is primarily hindered by the lack of suitable detection methods. Here we report a significant electrical magnetochiral anisotropy (EMCA) in an archetypal high-temperature cuprate superconductor NdBa2Cu3O7-δ, which is ascribed to the SOC effect under inversion and time-reversal symmetry violations in HTCS. Notably, a peculiar angular dependence of EMCA on the magnetic field orientation is observed, where an unprecedented higher-order EMCA effect is discovered. Based on Ginzburg-Landau theory analysis, the higher-order EMCA effect is intrinsically linked to magnetic-field-induced finite-momentum pairing states in HTCS. Our findings provide crucial insights into the exotic physics associated with SOC in HTCS, and pave the way for exploring high-temperature superconducting quantum electronics.