Patricia C. Marr, Andrew C. Marr
This opinion paper reflects upon highlights in ionic liquid (IL) gel research for green and sustainable chemistry. Discussed are some key observations from research into IL gels in catalysis, and insights into potential future uses and areas for development. It is noted that some IL gels have a remarkable ability to hold on to precious metals when used to entrap catalysts (nanoparticulate metals and complexes with minimal leaching) allowing heterogenized homogeneous catalysts to be reused, recycled and easily separated. Herein we present observations that IL gels can actively absorb and retain metals from solution. Evolving trends in research into liquids comprised of ions will be reviewed and a future in which the IL gels themselves are green and sustainable materials is hypothesized, which will accelerate their adoption as NaturIL gels in synthesis, materials, electronics and medicine. This article is part of the discussion meeting issue 'Ionic liquids and the future of soft materials'.