Efficient ammonia synthesis <i>via</i> electrocatalytic nitrate reduction over a [8 + 2]-connected three-dimensional metal-bipyridine covalent organic framework

Tsukasa Irie, Ayumu Kondo, Kai Sun, Kohki Sasaki, Mika Nozaki, Shiho Tomihari, Kotaro Sato, Tokuhisa Kawawaki, Yu Zhao, Saikat Das, Yuichi Negishi

原始摘要（英文原文）· Original abstract

TU-82, a 3D [8 + 2]-connected bcu COF, was post-synthetically metalated to yield TU-82-M ( M = Fe, Cu). TU-82-Fe shows outstanding activity and selectivity for electrocatalytic nitrate (NO 3 − ) reduction to ammonia via atomically dispersed Fe sites.

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Efficient ammonia synthesis <i>via</i> electrocatalytic nitrate reduction over a [8 + 2]-connected three-dimensional metal-bipyridine covalent organic framework

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