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◆ Chemical Science2025-11-03· Photon upconversion

Photon upconversion with indium phosphide quantum dots enables high-energy photoreactions using visible light

Indra Narayan Chakraborty, Adhra S. Sury, Aman Chaturvedi, Kaixing Wang, Ankit Dhankhar, Pankaj Mandal, Benjamin Dietzek‐Ivanšić, Pramod P. Pillai

原始摘要(英文原文)· Original abstract
the dehalogenation of substituted aryl halides in excellent yields. TTA-UC is the sole driving force for this photoredox reaction, as the required potential is beyond the maximum achievable redox potential of InP-QDs. Further, the scope of the QD-sensitized TTA-UC system is extended towards the radical polymerization of methyl methacrylate (MMA), resulting in the production of industrially important polymethyl methacrylate (PMMA). Our work overcomes key limitations of traditional UV-based photochemistry and introduces a sustainable, low-energy pathway for enabling high-energy transformations.
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Photon upconversion with indium phosphide quantum dots enables high-energy photoreactions using visible light — 科研速览 Science Skim