Long Chen, Wen‐Ping Zhang, Hao Tan, Yuping Zhang, Shuo Sun, Yancheng Zhu, Zhao‐Hua Yin, Hong Liu, Jianjun Wang
characterization, theoretical calculations, and performance evaluation, we further identify key future research directions, including multi-scale optimization of catalytic systems, electrolyzer design, and techno-economic analysis. This review aims to offer theoretical insights and practical guidance for the development of efficient, stable, and scalable electrocatalytic systems for green nitrile synthesis.