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◆ Journal of the American Chemical Society2026-05-14· Chemistry

Attenuating Imine Bond Polarization in Covalent Organic Frameworks Accelerates Charge and Proton Transport for High-Efficiency Photocatalytic Hydrogen Evolution

Zhipeng Luo, C W. LI, Wanxiang Yang, Yu Chang, Kai-Ling Wu, Liwei Xia, Jingru Gao, F Zhang, Qiwei Duan, Sibo Wang, Zailai Xie, Xiaofeng Wu, Guan‐E Wang, Wei Lin, Teng‐Teng Chen, Mingfei Zhou, Yihan Zhu, G Xu, Xiong Chen

原始摘要(英文原文)· Original abstract
and an apparent quantum yield of 21.8 ± 0.80% at 450 nm, vastly outperforming its neutral and electron-withdrawing counterparts. These mechanistic insights provide a dependable blueprint for the rational design of high-performance imine-linked COF photocatalysts.
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Attenuating Imine Bond Polarization in Covalent Organic Frameworks Accelerates Charge and Proton Transport for High-Efficiency Photocatalytic Hydrogen Evolution — 科研速览 Science Skim