Hai Zhu, Xinhao Peng, Jingyue Li, Shanshan Zhao, Yanzhuo Liu, Liangjian Zheng, Jia Fan, Huấn Cao, Jun Zhang, Shaobing Zhou
Despite established modalities such as chemotherapy and radiotherapy, cancer treatment remains hindered by off-target toxicity, drug resistance, and adverse effects. Cobalt-Based Biomaterials (Co-BMs) have emerged as versatile nanoplatforms for tumor theranostics, leveraging reversible Co 2+ /Co 3+ transitions to enable high-efficiency photothermal/photodynamic therapy, nanozyme catalysis, and reactive oxygen species (ROS) generation, supporting tumor microenvironment (TME) modulation and multimodal therapy. This review proposes a “structure-mechanism-translation” framework, systematically linking the physicochemical properties of Co-BMs with clinical needs, surpassing earlier reviews focused solely on synthesis or isolated applications. We describe the biological functions of Co-BMs ( e.g. , intracellular redox reactions, vitamin B12 synthesis, immune regulation, and cell proliferation and apoptosis), then overview current synthesis strategies for Co-BMs with diverse physicochemical characteristics ( e.g. , shape, surface modification, size), including template, etching, precipitation, sol-gel, hydro/solvothermal, and chemical vapor deposition methods. Furthermore, we highlight recent advances in multimodal tumor theranostics and microenvironment-responsive design, and critically examine key challenges. Finally, we discuss how current research informs future design principles to guide the development of next-generation multifunctional Co-BMs and advance their clinical translation in oncology.