Giulia Alice Volpato, Andrea Baciami, Kalina Georgieva Kjurchieva, Marco Berton, Marco Schiavon, Filippo Bano, Alessandra Ferrarini, Silvia Galvanin, Dario Mosconi, Juan Carlos Calderón, Silvia Pettenuzzo, Elena Colusso, Marco Roverso, Sara Bogialli, Elena Pastor, Laura Calvillo, Stefano Agnoli, Mattia Cattelan
In this work, we report a circular-economy approach to hydrogen production through the integration in an anion exchange membrane water electrolyzer (AEMWE) a nickel-based electrocatalyst prepared through circular recovery methods and hybridizing the electrolysis using urea oxidation. Ni(OH) 2 and NiO electrocatalysts are recovered from nickel-plating wastewater via a scalable hydrothermal synthesis. Urea, a common environmental pollutant, replaces the oxygen evolution reaction (OER) with urea oxidation, thereby reducing the overall energy demand. Hydrogen production using these circular catalysts and urea achieves performance comparable to benchmark nickel anodes at industrially relevant current densities, with a cell potential reduction of up to 0.25 V relative to OER. Gas chromatography, ion chromatography, and differential electrochemical mass spectrometry (DEMS) analyses identify N 2 and NO 2 − as the main nitrogen-containing products. Carbon adsorption species leads to partial deactivation during prolonged operation; however, the activity can be readily restored by polarity reversal or electrolyte switching. Finally, life cycle assessment (LCA) confirms that coupling urea oxidation with recycled nickel catalysts significantly lowers the CO 2 -equivalent footprint of hydrogen production, demonstrating the effectiveness of this circular and energy-efficient approach.