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◆ Chemical Engineering Journal2026-03-18· Backflow

On the importance of capillary-pressure gradient on water backflow during subsurface CO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" altimg="si58.svg" display="inline" id="d1e767"> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> </mml:msub> </mml:math> storage

Rouhi Farajzadeh, Vahid Niasar

原始摘要(英文原文)· Original abstract
Salt precipitation near the injection well is a major industrial challenge during CO 2 injection into saline aquifers, as it can severely reduce injectivity. This phenomenon has been attributed to strong capillary-driven backflow of brine towards the wellbore during the dry-out process. However, a widespread misconception holds that the absolute magnitude of capillary pressure controls the intensity of this backflow and the resulting salt accumulation. Using radial two-phase flow simulations with six bounded capillary-pressure–saturation functions, we demonstrate that it is the capillary-pressure gradient ( ∂ P c / ∂ x = ∂ P c / ∂ S w ⋅ ∂ S w / ∂ x ), not its absolute value, that governs water redistribution and backflow strength. Steeper gradients generate significantly stronger capillary forces, reverse brine flow near the dry-out front, enlarge the unsaturated zone, and slow front propagation. Critically, the most pronounced backflow and greatest potential for salt precipitation occur in systems with the largest | ∂ P c / ∂ S w | , even when capillary-pressure magnitudes differ substantially. These findings reveal that sharp contrasts in capillary-pressure gradients, caused by lithofacies transitions, layering, or material interfaces, can drive intense capillary fluxes across boundaries. Accurate characterization of gradient-dependent capillary behavior is therefore essential for reliably predicting injectivity impairment and salt-precipitation risks in geological CO 2 storage operations.
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On the importance of capillary-pressure gradient on water backflow during subsurface CO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" altimg="si58.svg" display="inline" id="d1e767"> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> </mml:msub> </mml:math> storage — 科研速览 Science Skim