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◆ Limnology and Oceanography Letters2025-11-29· Anaerobic oxidation of methane

Large methane oxidation across an oxygen gradient in Baltic Sea deep waters

Linnea Henriksson, Tristan McKenzie, Yvonne Y. Y. Yau, Henry L. S. Cheung, Claudia Majtényi‐Hill, Wilma Ljungberg, Aprajita S. Tomer, Stefano Bonaglia, Isaac R. Santos

原始摘要(英文原文)· Original abstract
Abstract Robust estimations of methane (CH 4 ) oxidation in marginal seas remain elusive, making CH 4 budgets particularly uncertain. Here, we investigate the CH 4 benthic source and bottom layer oxidation across the entire Baltic Sea using concentration and stable isotope (δ 13 C‐CH 4 ) profiles along oxygen and salinity gradients. CH 4 concentrations were highest near the seafloor under low oxygen conditions. Comparison with previous local‐scale studies implies increasing deep water CH 4 concentrations in the last decade. High CH 4 concentrations and δ 13 C‐CH 4 values (−54.4 ± 17.7‰) in bottom waters indicate benthic sources. Oxygen, salinity, and 224 Ra (benthic tracer) explained the CH 4 distribution. Methane oxidation estimated from δ 13 C‐CH 4 fractionation removed 49 ± 33% of benthic‐produced CH 4 before reaching the surface, leading to small water–air fluxes (10.0 ± 9.2 μ mol m −2 d −1 ). Overall, bottom layer CH 4 oxidation was highly effective attenuating CH 4 emissions to the atmosphere.
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